The quantification of material appearance is important in product design. In particular, the sparkle impression of metallic paint used mainly for automobiles varies with the observation angle. Although several evaluation methods and multi-angle measurement devices have been proposed for the impression, it is necessary to add more light sources or cameras to the devices to increase the number of evaluation angles. The present study constructed a device that evaluates the multi-angle sparkle impression in one shot and developed a method for quantifying the impression. The device comprises a line spectral camera, light source, and motorized rotation stage. The quantification method is based on spatial frequency characteristics. It was confirmed that the evaluation value obtained from the image recorded by the constructed device correlates closely with a subjective score. Furthermore, the evaluation value is significantly correlated with that obtained using a commercially available evaluation device.