In order to train a learning-based prediction model, large datasets are typically required. One of the major restrictions of machine learning applications using customized databases is the cost of human labor. In the previous papers [3, 4, 5], it is demonstrated through experiments that the correlation between thin-film nitrate sensor performance and surface texture exists. In the previous papers, several methods for extracting texture features from sensor images are explored, repeated cross-validation and a hyperparameter auto-tuning method are performed, and several machine learning models are built to improve prediction accuracy. In this paper, a new way to achieve the same accuracy with a much smaller dataset of labels by using an active learning structure is presented.